Articles | Volume 13, issue 5
https://doi.org/10.5194/os-13-649-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/os-13-649-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
04 Sep 2017
Research article |
| 04 Sep 2017
A measurement system for vertical seawater profiles close to the air–sea interface
Richard P. Sims
Plymouth Marine Laboratory, Plymouth, UK
University of Exeter, Exeter, UK
Ute Schuster
University of Exeter, Exeter, UK
Andrew J. Watson
University of Exeter, Exeter, UK
Ming Xi Yang
Plymouth Marine Laboratory, Plymouth, UK
Frances E. Hopkins
Plymouth Marine Laboratory, Plymouth, UK
John Stephens
Plymouth Marine Laboratory, Plymouth, UK
Plymouth Marine Laboratory, Plymouth, UK
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Sankirna D. Joge, Anoop S. Mahajan, Shrivardhan Hulswar, Christa A. Marandino, Martí Galí, Thomas G. Bell, and Rafel Simó
Biogeosciences, 21, 4439–4452, https://doi.org/10.5194/bg-21-4439-2024, https://doi.org/10.5194/bg-21-4439-2024, 2024
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Dimethyl sulfide (DMS) is the largest natural source of sulfur in the atmosphere and leads to the formation of cloud condensation nuclei. DMS emission and quantification of its impacts have large uncertainties, but a detailed study on the emissions and drivers of their uncertainty is missing to date. The emissions are usually calculated from the seawater DMS concentrations and a flux parameterization. Here we quantify the differences in DMS seawater products, which can affect DMS fluxes.
Sankirna D. Joge, Anoop S. Mahajan, Shrivardhan Hulswar, Christa A. Marandino, Martí Galí, Thomas G. Bell, Mingxi Yang, and Rafel Simó
Biogeosciences, 21, 4453–4467, https://doi.org/10.5194/bg-21-4453-2024, https://doi.org/10.5194/bg-21-4453-2024, 2024
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Dimethyl sulfide (DMS) is the largest natural source of sulfur in the atmosphere and leads to the formation of cloud condensation nuclei. DMS emissions and quantification of their impacts have large uncertainties, but a detailed study on the range of emissions and drivers of their uncertainty is missing to date. The emissions are calculated from the seawater DMS concentrations and a flux parameterization. Here we quantify the differences in the effect of flux parameterizations used in models.
Neill Mackay, Taimoor Sohail, Jan David Zika, Richard G. Williams, Oliver Andrews, and Andrew James Watson
Geosci. Model Dev., 17, 5987–6005, https://doi.org/10.5194/gmd-17-5987-2024, https://doi.org/10.5194/gmd-17-5987-2024, 2024
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The ocean absorbs carbon dioxide from the atmosphere, mitigating climate change, but estimates of the uptake do not always agree. There is a need to reconcile these differing estimates and to improve our understanding of ocean carbon uptake. We present a new method for estimating ocean carbon uptake and test it with model data. The method effectively diagnoses the ocean carbon uptake from limited data and therefore shows promise for reconciling different observational estimates.
Alexander T. Archibald, Bablu Sinha, Maria Russo, Emily Matthews, Freya Squires, N. Luke Abraham, Stephane Bauguitte, Thomas Bannan, Thomas Bell, David Berry, Lucy Carpenter, Hugh Coe, Andrew Coward, Peter Edwards, Daniel Feltham, Dwayne Heard, Jim Hopkins, James Keeble, Elizabeth C. Kent, Brian King, Isobel R. Lawrence, James Lee, Claire R. Macintosh, Alex Megann, Ben I. Moat, Katie Read, Chris Reed, Malcolm Roberts, Reinhard Schiemann, David Schroeder, Tim Smyth, Loren Temple, Navaneeth Thamban, Lisa Whalley, Simon Williams, Huihui Wu, and Ming-Xi Yang
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-405, https://doi.org/10.5194/essd-2023-405, 2024
Revised manuscript accepted for ESSD
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Here we present an overview of the data generated as part of the North Atlantic Climate System Integrated Studies (ACSIS) programme which are available through dedicated repositories at the Centre for Environmental Data Analysis (CEDA, www.ceda.ac.uk) and the British Oceanographic Data Centre (BODC, bodc.ac.uk). ACSIS data cover the full North Atlantic System comprising: the North Atlantic Ocean, the atmosphere above it including its composition, Arctic Sea Ice and the Greenland Ice Sheet.
George Manville, Thomas G. Bell, Jane P. Mulcahy, Rafel Simó, Martí Galí, Anoop S. Mahajan, Shrivardhan Hulswar, and Paul R. Halloran
Biogeosciences, 20, 1813–1828, https://doi.org/10.5194/bg-20-1813-2023, https://doi.org/10.5194/bg-20-1813-2023, 2023
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We present the first global investigation of controls on seawater dimethylsulfide (DMS) spatial variability over scales of up to 100 km. Sea surface height anomalies, density, and chlorophyll a help explain almost 80 % of DMS variability. The results suggest that physical and biogeochemical processes play an equally important role in controlling DMS variability. These data provide independent confirmation that existing parameterisations of seawater DMS concentration use appropriate variables.
Veronica Z. Berta, Lynn M. Russell, Derek J. Price, Chia-Li Chen, Alex K. Y. Lee, Patricia K. Quinn, Timothy S. Bates, Thomas G. Bell, and Michael J. Behrenfeld
Atmos. Chem. Phys., 23, 2765–2787, https://doi.org/10.5194/acp-23-2765-2023, https://doi.org/10.5194/acp-23-2765-2023, 2023
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Amines are compounds emitted from a variety of marine and continental sources and were measured by aerosol mass spectrometry and Fourier transform infrared spectroscopy during the North Atlantic Aerosols and Marine Ecosystems Study (NAAMES) cruises. Secondary continental and primary marine sources of amines were identified by comparisons to tracers. The results show that the two methods are complementary for investigating amines in the marine environment.
Shrivardhan Hulswar, Rafel Simó, Martí Galí, Thomas G. Bell, Arancha Lana, Swaleha Inamdar, Paul R. Halloran, George Manville, and Anoop Sharad Mahajan
Earth Syst. Sci. Data, 14, 2963–2987, https://doi.org/10.5194/essd-14-2963-2022, https://doi.org/10.5194/essd-14-2963-2022, 2022
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The third climatological estimation of sea surface dimethyl sulfide (DMS) concentrations based on in situ measurements was created (DMS-Rev3). The update includes a much larger input dataset and includes improvements in the data unification, filtering, and smoothing algorithm. The DMS-Rev3 climatology provides more realistic monthly estimates of DMS, and shows significant regional differences compared to past climatologies.
Pierre Friedlingstein, Matthew W. Jones, Michael O'Sullivan, Robbie M. Andrew, Dorothee C. E. Bakker, Judith Hauck, Corinne Le Quéré, Glen P. Peters, Wouter Peters, Julia Pongratz, Stephen Sitch, Josep G. Canadell, Philippe Ciais, Rob B. Jackson, Simone R. Alin, Peter Anthoni, Nicholas R. Bates, Meike Becker, Nicolas Bellouin, Laurent Bopp, Thi Tuyet Trang Chau, Frédéric Chevallier, Louise P. Chini, Margot Cronin, Kim I. Currie, Bertrand Decharme, Laique M. Djeutchouang, Xinyu Dou, Wiley Evans, Richard A. Feely, Liang Feng, Thomas Gasser, Dennis Gilfillan, Thanos Gkritzalis, Giacomo Grassi, Luke Gregor, Nicolas Gruber, Özgür Gürses, Ian Harris, Richard A. Houghton, George C. Hurtt, Yosuke Iida, Tatiana Ilyina, Ingrid T. Luijkx, Atul Jain, Steve D. Jones, Etsushi Kato, Daniel Kennedy, Kees Klein Goldewijk, Jürgen Knauer, Jan Ivar Korsbakken, Arne Körtzinger, Peter Landschützer, Siv K. Lauvset, Nathalie Lefèvre, Sebastian Lienert, Junjie Liu, Gregg Marland, Patrick C. McGuire, Joe R. Melton, David R. Munro, Julia E. M. S. Nabel, Shin-Ichiro Nakaoka, Yosuke Niwa, Tsuneo Ono, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Thais M. Rosan, Jörg Schwinger, Clemens Schwingshackl, Roland Séférian, Adrienne J. Sutton, Colm Sweeney, Toste Tanhua, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Francesco Tubiello, Guido R. van der Werf, Nicolas Vuichard, Chisato Wada, Rik Wanninkhof, Andrew J. Watson, David Willis, Andrew J. Wiltshire, Wenping Yuan, Chao Yue, Xu Yue, Sönke Zaehle, and Jiye Zeng
Earth Syst. Sci. Data, 14, 1917–2005, https://doi.org/10.5194/essd-14-1917-2022, https://doi.org/10.5194/essd-14-1917-2022, 2022
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The Global Carbon Budget 2021 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Richard P. Sims, Michael Bedington, Ute Schuster, Andrew J. Watson, Vassilis Kitidis, Ricardo Torres, Helen S. Findlay, James R. Fishwick, Ian Brown, and Thomas G. Bell
Biogeosciences, 19, 1657–1674, https://doi.org/10.5194/bg-19-1657-2022, https://doi.org/10.5194/bg-19-1657-2022, 2022
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The amount of carbon dioxide (CO2) being absorbed by the ocean is relevant to the earth's climate. CO2 values in the coastal ocean and estuaries are not well known because of the instrumentation used. We used a new approach to measure CO2 across the coastal and estuarine zone. We found that CO2 and salinity were linked to the state of the tide. We used our CO2 measurements and model salinity to predict CO2. Previous studies overestimate how much CO2 the coastal ocean draws down at our site.
Kevin J. Sanchez, Bo Zhang, Hongyu Liu, Matthew D. Brown, Ewan C. Crosbie, Francesca Gallo, Johnathan W. Hair, Chris A. Hostetler, Carolyn E. Jordan, Claire E. Robinson, Amy Jo Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Elizabeth B. Wiggins, Edward L. Winstead, Luke D. Ziemba, Georges Saliba, Savannah L. Lewis, Lynn M. Russell, Patricia K. Quinn, Timothy S. Bates, Jack Porter, Thomas G. Bell, Peter Gaube, Eric S. Saltzman, Michael J. Behrenfeld, and Richard H. Moore
Atmos. Chem. Phys., 22, 2795–2815, https://doi.org/10.5194/acp-22-2795-2022, https://doi.org/10.5194/acp-22-2795-2022, 2022
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Atmospheric particle concentrations impact clouds, which strongly impact the amount of sunlight reflected back into space and the overall climate. Measurements of particles over the ocean are rare and expensive to collect, so models are necessary to fill in the gaps by simulating both particle and clouds. However, some measurements are needed to test the accuracy of the models. Here, we measure changes in particles in different weather conditions, which are ideal for comparison with models.
Zhaohui Chen, Parvadha Suntharalingam, Andrew J. Watson, Ute Schuster, Jiang Zhu, and Ning Zeng
Biogeosciences, 18, 4549–4570, https://doi.org/10.5194/bg-18-4549-2021, https://doi.org/10.5194/bg-18-4549-2021, 2021
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As the global temperature continues to increase, carbon dioxide (CO2) is a major driver of this global warming. The increased CO2 is mainly caused by emissions from fossil fuel use and land use. At the same time, the ocean is a significant sink in the carbon cycle. The North Atlantic is a critical ocean region in reducing CO2 concentration. We estimate the CO2 uptake in this region based on a carbon inverse system and atmospheric CO2 observations.
Daniel P. Phillips, Frances E. Hopkins, Thomas G. Bell, Peter S. Liss, Philip D. Nightingale, Claire E. Reeves, Charel Wohl, and Mingxi Yang
Atmos. Chem. Phys., 21, 10111–10132, https://doi.org/10.5194/acp-21-10111-2021, https://doi.org/10.5194/acp-21-10111-2021, 2021
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We present the first measurements of the rate of transfer (flux) of three gases between the atmosphere and the ocean, using a direct flux measurement technique, at a coastal site. We show greater atmospheric loss of acetone and acetaldehyde into the ocean than estimated by global models for the open water; importantly, the acetaldehyde transfer direction is opposite to the model estimates. Measured dimethylsulfide fluxes agreed with a recent model. Isoprene fluxes were too weak to be measured.
Yuanxu Dong, Mingxi Yang, Dorothee C. E. Bakker, Vassilis Kitidis, and Thomas G. Bell
Atmos. Chem. Phys., 21, 8089–8110, https://doi.org/10.5194/acp-21-8089-2021, https://doi.org/10.5194/acp-21-8089-2021, 2021
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Eddy covariance (EC) is the most direct method for measuring air–sea CO2 flux from ships. However, uncertainty in EC air–sea CO2 fluxes has not been well quantified. Here we show that with the state-of-the-art gas analysers, instrumental noise no longer contributes significantly to the CO2 flux uncertainty. Applying an appropriate averaging timescale (1–3 h) and suitable air–sea CO2 fugacity threshold (at least 20 µatm) to EC flux data enables an optimal analysis of the gas transfer velocity.
Kevin J. Sanchez, Bo Zhang, Hongyu Liu, Georges Saliba, Chia-Li Chen, Savannah L. Lewis, Lynn M. Russell, Michael A. Shook, Ewan C. Crosbie, Luke D. Ziemba, Matthew D. Brown, Taylor J. Shingler, Claire E. Robinson, Elizabeth B. Wiggins, Kenneth L. Thornhill, Edward L. Winstead, Carolyn Jordan, Patricia K. Quinn, Timothy S. Bates, Jack Porter, Thomas G. Bell, Eric S. Saltzman, Michael J. Behrenfeld, and Richard H. Moore
Atmos. Chem. Phys., 21, 831–851, https://doi.org/10.5194/acp-21-831-2021, https://doi.org/10.5194/acp-21-831-2021, 2021
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Models describing atmospheric airflow were combined with satellite measurements representative of marine phytoplankton and other meteorological variables. These combined variables were compared to measured aerosol to identify upwind influences on aerosol concentrations. Results indicate that phytoplankton production rates upwind impact the aerosol mass. Also, results suggest that the condensation of mass onto short-lived large sea spray particles may be a significant sink of aerosol mass.
David C. Loades, Mingxi Yang, Thomas G. Bell, Adam R. Vaughan, Ryan J. Pound, Stefan Metzger, James D. Lee, and Lucy J. Carpenter
Atmos. Meas. Tech., 13, 6915–6931, https://doi.org/10.5194/amt-13-6915-2020, https://doi.org/10.5194/amt-13-6915-2020, 2020
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The loss of ozone to the sea surface was measured from the south coast of the UK and was found to be more rapid than previous observations over the open ocean. This is likely a consequence of different chemistry and biology in coastal environments. Strong winds appeared to speed up the loss of ozone. A better understanding of what influences ozone loss over the sea will lead to better model estimates of total ozone in the troposphere.
Pierre Friedlingstein, Michael O'Sullivan, Matthew W. Jones, Robbie M. Andrew, Judith Hauck, Are Olsen, Glen P. Peters, Wouter Peters, Julia Pongratz, Stephen Sitch, Corinne Le Quéré, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Simone Alin, Luiz E. O. C. Aragão, Almut Arneth, Vivek Arora, Nicholas R. Bates, Meike Becker, Alice Benoit-Cattin, Henry C. Bittig, Laurent Bopp, Selma Bultan, Naveen Chandra, Frédéric Chevallier, Louise P. Chini, Wiley Evans, Liesbeth Florentie, Piers M. Forster, Thomas Gasser, Marion Gehlen, Dennis Gilfillan, Thanos Gkritzalis, Luke Gregor, Nicolas Gruber, Ian Harris, Kerstin Hartung, Vanessa Haverd, Richard A. Houghton, Tatiana Ilyina, Atul K. Jain, Emilie Joetzjer, Koji Kadono, Etsushi Kato, Vassilis Kitidis, Jan Ivar Korsbakken, Peter Landschützer, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Zhu Liu, Danica Lombardozzi, Gregg Marland, Nicolas Metzl, David R. Munro, Julia E. M. S. Nabel, Shin-Ichiro Nakaoka, Yosuke Niwa, Kevin O'Brien, Tsuneo Ono, Paul I. Palmer, Denis Pierrot, Benjamin Poulter, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Adam J. P. Smith, Adrienne J. Sutton, Toste Tanhua, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Guido van der Werf, Nicolas Vuichard, Anthony P. Walker, Rik Wanninkhof, Andrew J. Watson, David Willis, Andrew J. Wiltshire, Wenping Yuan, Xu Yue, and Sönke Zaehle
Earth Syst. Sci. Data, 12, 3269–3340, https://doi.org/10.5194/essd-12-3269-2020, https://doi.org/10.5194/essd-12-3269-2020, 2020
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The Global Carbon Budget 2020 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Wei-Lei Wang, Guisheng Song, François Primeau, Eric S. Saltzman, Thomas G. Bell, and J. Keith Moore
Biogeosciences, 17, 5335–5354, https://doi.org/10.5194/bg-17-5335-2020, https://doi.org/10.5194/bg-17-5335-2020, 2020
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Dimethyl sulfide, a volatile compound produced as a byproduct of marine phytoplankton activity, can be emitted to the atmosphere via gas exchange. In the atmosphere, DMS is oxidized to cloud condensation nuclei, thus contributing to cloud formation. Therefore, oceanic DMS plays an important role in regulating the planet's climate by influencing the radiation budget. In this study, we use an artificial neural network model to update the global DMS climatology and estimate the sea-to-air flux.
Sarah J. Lawson, Cliff S. Law, Mike J. Harvey, Thomas G. Bell, Carolyn F. Walker, Warren J. de Bruyn, and Eric S. Saltzman
Atmos. Chem. Phys., 20, 3061–3078, https://doi.org/10.5194/acp-20-3061-2020, https://doi.org/10.5194/acp-20-3061-2020, 2020
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Methanethiol (MeSH) is a reduced sulfur gas originating from phytoplankton, with a global ocean source of ~ 17 % of dimethyl sulfide (DMS). It has been little studied and is rarely observed over the ocean. In this work, MeSH was measured at much higher levels than previously observed (3–36 % of parallel DMS mixing ratios). MeSH could be a significant source of atmospheric sulfur over productive regions of the ocean, but its distribution, and its atmospheric impact, requires more investigation.
Jan D. Zika, Jean-Baptiste Sallée, Andrew J. S. Meijers, Alberto C. Naveira-Garabato, Andrew J. Watson, Marie-Jose Messias, and Brian A. King
Ocean Sci., 16, 323–336, https://doi.org/10.5194/os-16-323-2020, https://doi.org/10.5194/os-16-323-2020, 2020
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The ocean can regulate climate by distributing heat and carbon dioxide into its interior. This work has resulted from a major experiment aimed at understanding how that distribution occurs. In the experiment an artificial tracer was released into the ocean. After release the tracer was tracked as it was distorted by ocean currents. Using novel methods we reveal how the tracer's distortions follow the movement of the underlying water masses in the ocean and we estimate the rate at which it mixes.
Frances E. Hopkins, Philip D. Nightingale, John A. Stephens, C. Mark Moore, Sophie Richier, Gemma L. Cripps, and Stephen D. Archer
Biogeosciences, 17, 163–186, https://doi.org/10.5194/bg-17-163-2020, https://doi.org/10.5194/bg-17-163-2020, 2020
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We investigated the effects of ocean acidification (OA) on the production of climate active gas dimethylsulfide (DMS) in polar waters. We found that polar DMS production was unaffected by OA – in contrast to temperate waters, where large increases in DMS occurred. The regional differences in DMS response may reflect natural variability in community adaptation to ambient carbonate chemistry and should be taken into account in predicting the influence of future DMS emissions on Earth's climate.
Mingxi Yang, Sarah J. Norris, Thomas G. Bell, and Ian M. Brooks
Atmos. Chem. Phys., 19, 15271–15284, https://doi.org/10.5194/acp-19-15271-2019, https://doi.org/10.5194/acp-19-15271-2019, 2019
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This work reports direct measurements of sea spray fluxes from a coastal site in the UK, which are relevant for atmospheric chemistry as well as coastal air quality. Sea spray fluxes from this location are roughly an order of magnitude greater than over the open ocean at similar wind conditions, comparable to previous coastal measurements. Unlike previous open ocean measurements that are largely wind speed dependent, we find that sea spray fluxes near the coast depend more strongly on waves.
Mingxi Yang, Thomas G. Bell, Ian J. Brown, James R. Fishwick, Vassilis Kitidis, Philip D. Nightingale, Andrew P. Rees, and Timothy J. Smyth
Biogeosciences, 16, 961–978, https://doi.org/10.5194/bg-16-961-2019, https://doi.org/10.5194/bg-16-961-2019, 2019
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We quantify the emissions and uptake of the greenhouse gases carbon dioxide and methane from the coastal seas of the UK over 1 year using the state-of-the-art eddy covariance technique. Our measurements show how these air–sea fluxes vary twice a day (tidal), diurnally (circadian) and seasonally. We also estimate the air–sea gas transfer velocity, which is essential for modelling and predicting coastal air-sea exchange.
Corinne Le Quéré, Robbie M. Andrew, Pierre Friedlingstein, Stephen Sitch, Judith Hauck, Julia Pongratz, Penelope A. Pickers, Jan Ivar Korsbakken, Glen P. Peters, Josep G. Canadell, Almut Arneth, Vivek K. Arora, Leticia Barbero, Ana Bastos, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Philippe Ciais, Scott C. Doney, Thanos Gkritzalis, Daniel S. Goll, Ian Harris, Vanessa Haverd, Forrest M. Hoffman, Mario Hoppema, Richard A. Houghton, George Hurtt, Tatiana Ilyina, Atul K. Jain, Truls Johannessen, Chris D. Jones, Etsushi Kato, Ralph F. Keeling, Kees Klein Goldewijk, Peter Landschützer, Nathalie Lefèvre, Sebastian Lienert, Zhu Liu, Danica Lombardozzi, Nicolas Metzl, David R. Munro, Julia E. M. S. Nabel, Shin-ichiro Nakaoka, Craig Neill, Are Olsen, Tsueno Ono, Prabir Patra, Anna Peregon, Wouter Peters, Philippe Peylin, Benjamin Pfeil, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Laure Resplandy, Eddy Robertson, Matthias Rocher, Christian Rödenbeck, Ute Schuster, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Tobias Steinhoff, Adrienne Sutton, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Francesco N. Tubiello, Ingrid T. van der Laan-Luijkx, Guido R. van der Werf, Nicolas Viovy, Anthony P. Walker, Andrew J. Wiltshire, Rebecca Wright, Sönke Zaehle, and Bo Zheng
Earth Syst. Sci. Data, 10, 2141–2194, https://doi.org/10.5194/essd-10-2141-2018, https://doi.org/10.5194/essd-10-2141-2018, 2018
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The Global Carbon Budget 2018 describes the data sets and methodology used to quantify the emissions of carbon dioxide and their partitioning among the atmosphere, land, and ocean. These living data are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Murray J. Smith, Carolyn F. Walker, Thomas G. Bell, Mike J. Harvey, Eric S. Saltzman, and Cliff S. Law
Atmos. Chem. Phys., 18, 5861–5877, https://doi.org/10.5194/acp-18-5861-2018, https://doi.org/10.5194/acp-18-5861-2018, 2018
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The transfer of gases across the air–sea interface has a significant influence on climate. During a research voyage in the South Pacific we measured the transfer rate of the biogenic gas dimethyl sulfide (DMS) from the ocean using two independent methods. The agreement between the techniques provides confidence in their use in compilations of global gas transfer. We also identified physical conditions under which the observations are not well predicted by a standard gas transfer model.
Sebastian Landwehr, Scott D. Miller, Murray J. Smith, Thomas G. Bell, Eric S. Saltzman, and Brian Ward
Atmos. Chem. Phys., 18, 4297–4315, https://doi.org/10.5194/acp-18-4297-2018, https://doi.org/10.5194/acp-18-4297-2018, 2018
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The ocean takes up about 25 % of emitted anthropogenic emitted carbon dioxide and thus plays a significant role in the regulation of climate. In order to accurately calculate this uptake, a quantity known as the air–sea gas transfer velocity needs to be determined. This is typically parameterised with mean wind speed, the most commonly used velocity scale for calculating air–sea transfer coefficients. In this article, we propose an alternative velocity scale known as the friction velocity.
Corinne Le Quéré, Robbie M. Andrew, Pierre Friedlingstein, Stephen Sitch, Julia Pongratz, Andrew C. Manning, Jan Ivar Korsbakken, Glen P. Peters, Josep G. Canadell, Robert B. Jackson, Thomas A. Boden, Pieter P. Tans, Oliver D. Andrews, Vivek K. Arora, Dorothee C. E. Bakker, Leticia Barbero, Meike Becker, Richard A. Betts, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Philippe Ciais, Catherine E. Cosca, Jessica Cross, Kim Currie, Thomas Gasser, Ian Harris, Judith Hauck, Vanessa Haverd, Richard A. Houghton, Christopher W. Hunt, George Hurtt, Tatiana Ilyina, Atul K. Jain, Etsushi Kato, Markus Kautz, Ralph F. Keeling, Kees Klein Goldewijk, Arne Körtzinger, Peter Landschützer, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Ivan Lima, Danica Lombardozzi, Nicolas Metzl, Frank Millero, Pedro M. S. Monteiro, David R. Munro, Julia E. M. S. Nabel, Shin-ichiro Nakaoka, Yukihiro Nojiri, X. Antonio Padin, Anna Peregon, Benjamin Pfeil, Denis Pierrot, Benjamin Poulter, Gregor Rehder, Janet Reimer, Christian Rödenbeck, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Benjamin D. Stocker, Hanqin Tian, Bronte Tilbrook, Francesco N. Tubiello, Ingrid T. van der Laan-Luijkx, Guido R. van der Werf, Steven van Heuven, Nicolas Viovy, Nicolas Vuichard, Anthony P. Walker, Andrew J. Watson, Andrew J. Wiltshire, Sönke Zaehle, and Dan Zhu
Earth Syst. Sci. Data, 10, 405–448, https://doi.org/10.5194/essd-10-405-2018, https://doi.org/10.5194/essd-10-405-2018, 2018
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The Global Carbon Budget 2017 describes data sets and methodology to quantify the five major components of the global carbon budget and their uncertainties. It is the 12th annual update and the 6th published in this journal.
Cliff S. Law, Murray J. Smith, Mike J. Harvey, Thomas G. Bell, Luke T. Cravigan, Fiona C. Elliott, Sarah J. Lawson, Martine Lizotte, Andrew Marriner, John McGregor, Zoran Ristovski, Karl A. Safi, Eric S. Saltzman, Petri Vaattovaara, and Carolyn F. Walker
Atmos. Chem. Phys., 17, 13645–13667, https://doi.org/10.5194/acp-17-13645-2017, https://doi.org/10.5194/acp-17-13645-2017, 2017
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We carried out a multidisciplinary study to examine how aerosol production is influenced by the production and emission of trace gases and particles in the surface ocean. Phytoplankton blooms of different species composition in frontal waters southeast of New Zealand were a significant source of dimethylsulfide and other aerosol precursors. The relationships between surface ocean biogeochemistry and aerosol composition will inform the understanding of aerosol production over the remote ocean.
Thomas G. Bell, Sebastian Landwehr, Scott D. Miller, Warren J. de Bruyn, Adrian H. Callaghan, Brian Scanlon, Brian Ward, Mingxi Yang, and Eric S. Saltzman
Atmos. Chem. Phys., 17, 9019–9033, https://doi.org/10.5194/acp-17-9019-2017, https://doi.org/10.5194/acp-17-9019-2017, 2017
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The mechanisms that determine the air–sea exchange of gases such as carbon dioxide are not well understood. During a research cruise in the North Atlantic, we simultaneously measured the air–sea transfer of two gases with contrasting solubility over a range in wind and wave conditions. We compare the transfer of these gases to improve understanding of how bubbles from breaking waves may mediate air–sea gas fluxes.
Mingxi Yang, John Prytherch, Elena Kozlova, Margaret J. Yelland, Deepulal Parenkat Mony, and Thomas G. Bell
Atmos. Meas. Tech., 9, 5509–5522, https://doi.org/10.5194/amt-9-5509-2016, https://doi.org/10.5194/amt-9-5509-2016, 2016
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The exchange of the greenhouse gases carbon dioxide and methane between the ocean and the atmosphere is of critical importance for the earth's climate. Despite this, direct measurements of these fluxes are relatively scarce, especially for methane, in large part due to instrumental challenges. In this paper, we evaluate the performance of two of the latest carbon dioxide and methane flux analysers. We also compare their detection limits to predicted air–sea fluxes of these gases.
Corinne Le Quéré, Robbie M. Andrew, Josep G. Canadell, Stephen Sitch, Jan Ivar Korsbakken, Glen P. Peters, Andrew C. Manning, Thomas A. Boden, Pieter P. Tans, Richard A. Houghton, Ralph F. Keeling, Simone Alin, Oliver D. Andrews, Peter Anthoni, Leticia Barbero, Laurent Bopp, Frédéric Chevallier, Louise P. Chini, Philippe Ciais, Kim Currie, Christine Delire, Scott C. Doney, Pierre Friedlingstein, Thanos Gkritzalis, Ian Harris, Judith Hauck, Vanessa Haverd, Mario Hoppema, Kees Klein Goldewijk, Atul K. Jain, Etsushi Kato, Arne Körtzinger, Peter Landschützer, Nathalie Lefèvre, Andrew Lenton, Sebastian Lienert, Danica Lombardozzi, Joe R. Melton, Nicolas Metzl, Frank Millero, Pedro M. S. Monteiro, David R. Munro, Julia E. M. S. Nabel, Shin-ichiro Nakaoka, Kevin O'Brien, Are Olsen, Abdirahman M. Omar, Tsuneo Ono, Denis Pierrot, Benjamin Poulter, Christian Rödenbeck, Joe Salisbury, Ute Schuster, Jörg Schwinger, Roland Séférian, Ingunn Skjelvan, Benjamin D. Stocker, Adrienne J. Sutton, Taro Takahashi, Hanqin Tian, Bronte Tilbrook, Ingrid T. van der Laan-Luijkx, Guido R. van der Werf, Nicolas Viovy, Anthony P. Walker, Andrew J. Wiltshire, and Sönke Zaehle
Earth Syst. Sci. Data, 8, 605–649, https://doi.org/10.5194/essd-8-605-2016, https://doi.org/10.5194/essd-8-605-2016, 2016
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The Global Carbon Budget 2016 is the 11th annual update of emissions of carbon dioxide (CO2) and their partitioning among the atmosphere, land, and ocean. This data synthesis brings together measurements, statistical information, and analyses of model results in order to provide an assessment of the global carbon budget and their uncertainties for years 1959 to 2015, with a projection for year 2016.
Dorothee C. E. Bakker, Benjamin Pfeil, Camilla S. Landa, Nicolas Metzl, Kevin M. O'Brien, Are Olsen, Karl Smith, Cathy Cosca, Sumiko Harasawa, Stephen D. Jones, Shin-ichiro Nakaoka, Yukihiro Nojiri, Ute Schuster, Tobias Steinhoff, Colm Sweeney, Taro Takahashi, Bronte Tilbrook, Chisato Wada, Rik Wanninkhof, Simone R. Alin, Carlos F. Balestrini, Leticia Barbero, Nicholas R. Bates, Alejandro A. Bianchi, Frédéric Bonou, Jacqueline Boutin, Yann Bozec, Eugene F. Burger, Wei-Jun Cai, Robert D. Castle, Liqi Chen, Melissa Chierici, Kim Currie, Wiley Evans, Charles Featherstone, Richard A. Feely, Agneta Fransson, Catherine Goyet, Naomi Greenwood, Luke Gregor, Steven Hankin, Nick J. Hardman-Mountford, Jérôme Harlay, Judith Hauck, Mario Hoppema, Matthew P. Humphreys, Christopher W. Hunt, Betty Huss, J. Severino P. Ibánhez, Truls Johannessen, Ralph Keeling, Vassilis Kitidis, Arne Körtzinger, Alex Kozyr, Evangelia Krasakopoulou, Akira Kuwata, Peter Landschützer, Siv K. Lauvset, Nathalie Lefèvre, Claire Lo Monaco, Ansley Manke, Jeremy T. Mathis, Liliane Merlivat, Frank J. Millero, Pedro M. S. Monteiro, David R. Munro, Akihiko Murata, Timothy Newberger, Abdirahman M. Omar, Tsuneo Ono, Kristina Paterson, David Pearce, Denis Pierrot, Lisa L. Robbins, Shu Saito, Joe Salisbury, Reiner Schlitzer, Bernd Schneider, Roland Schweitzer, Rainer Sieger, Ingunn Skjelvan, Kevin F. Sullivan, Stewart C. Sutherland, Adrienne J. Sutton, Kazuaki Tadokoro, Maciej Telszewski, Matthias Tuma, Steven M. A. C. van Heuven, Doug Vandemark, Brian Ward, Andrew J. Watson, and Suqing Xu
Earth Syst. Sci. Data, 8, 383–413, https://doi.org/10.5194/essd-8-383-2016, https://doi.org/10.5194/essd-8-383-2016, 2016
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Version 3 of the Surface Ocean CO2 Atlas (www.socat.info) has 14.5 million CO2 (carbon dioxide) values for the years 1957 to 2014 covering the global oceans and coastal seas. Version 3 is an update to version 2 with a longer record and 44 % more CO2 values. The CO2 measurements have been made on ships, fixed moorings and drifting buoys. SOCAT enables quantification of the ocean carbon sink and ocean acidification, as well as model evaluation, thus informing climate negotiations.
Carolyn F. Walker, Mike J. Harvey, Murray J. Smith, Thomas G. Bell, Eric S. Saltzman, Andrew S. Marriner, John A. McGregor, and Cliff S. Law
Ocean Sci., 12, 1033–1048, https://doi.org/10.5194/os-12-1033-2016, https://doi.org/10.5194/os-12-1033-2016, 2016
Alison L. Webb, Emma Leedham-Elvidge, Claire Hughes, Frances E. Hopkins, Gill Malin, Lennart T. Bach, Kai Schulz, Kate Crawfurd, Corina P. D. Brussaard, Annegret Stuhr, Ulf Riebesell, and Peter S. Liss
Biogeosciences, 13, 4595–4613, https://doi.org/10.5194/bg-13-4595-2016, https://doi.org/10.5194/bg-13-4595-2016, 2016
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This paper presents concentrations of several trace gases produced by the Baltic Sea phytoplankton community during a mesocosm experiment with five different CO2 levels. Average concentrations of dimethylsulphide were lower in the highest CO2 mesocosms over a 6-week period, corresponding to previous mesocosm experiment results. No dimethylsulfoniopropionate was detected due to a methodological issue. Concentrations of iodine- and bromine-containing halocarbons were unaffected by increasing CO2.
Mingxi Yang, Thomas G. Bell, Frances E. Hopkins, Vassilis Kitidis, Pierre W. Cazenave, Philip D. Nightingale, Margaret J. Yelland, Robin W. Pascal, John Prytherch, Ian M. Brooks, and Timothy J. Smyth
Atmos. Chem. Phys., 16, 5745–5761, https://doi.org/10.5194/acp-16-5745-2016, https://doi.org/10.5194/acp-16-5745-2016, 2016
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Coastal seas are sources of methane in the atmosphere and can fluctuate from emitting to absorbing carbon dioxide. Direct air–sea transport measurements of these two greenhouse gases in near shore regions remain scarce. From a recently established coastal atmospheric station on the south-west coast of the UK, we observed that the oceanic absorption of carbon dioxide peaked during the phytoplankton bloom, while methane emission varied with the tidal cycle, likely due to an estuary influence.
Mingxi Yang, Thomas G. Bell, Frances E. Hopkins, and Timothy J. Smyth
Atmos. Chem. Phys., 16, 4771–4783, https://doi.org/10.5194/acp-16-4771-2016, https://doi.org/10.5194/acp-16-4771-2016, 2016
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Exhausts from ships are an important source of air pollution in coastal regions. We observed a ~ 3 fold reduction in the level of sulfur dioxide (a principle pollutant) from the English Channel from 2014 to 2015 after the new International Maritime Organisation regulation on ship sulfur emission became law. Our estimated ship's fuel sulfur content shows a high degree of compliance. Dimethylsulfide from the marine biota becomes a relatively more important source of sulfur in coastal marine air.
C. Rödenbeck, D. C. E. Bakker, N. Gruber, Y. Iida, A. R. Jacobson, S. Jones, P. Landschützer, N. Metzl, S. Nakaoka, A. Olsen, G.-H. Park, P. Peylin, K. B. Rodgers, T. P. Sasse, U. Schuster, J. D. Shutler, V. Valsala, R. Wanninkhof, and J. Zeng
Biogeosciences, 12, 7251–7278, https://doi.org/10.5194/bg-12-7251-2015, https://doi.org/10.5194/bg-12-7251-2015, 2015
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This study investigates variations in the CO2 uptake of the ocean from year to year. These variations have been calculated from measurements of the surface-ocean carbon content by various different interpolation methods. The equatorial Pacific is estimated to be the region with the strongest year-to-year variations, tied to the El Nino phase. The global ocean CO2 uptake gradually increased from about the year 2000. The comparison of the interpolation methods identifies these findings as robust.
C. Le Quéré, R. Moriarty, R. M. Andrew, J. G. Canadell, S. Sitch, J. I. Korsbakken, P. Friedlingstein, G. P. Peters, R. J. Andres, T. A. Boden, R. A. Houghton, J. I. House, R. F. Keeling, P. Tans, A. Arneth, D. C. E. Bakker, L. Barbero, L. Bopp, J. Chang, F. Chevallier, L. P. Chini, P. Ciais, M. Fader, R. A. Feely, T. Gkritzalis, I. Harris, J. Hauck, T. Ilyina, A. K. Jain, E. Kato, V. Kitidis, K. Klein Goldewijk, C. Koven, P. Landschützer, S. K. Lauvset, N. Lefèvre, A. Lenton, I. D. Lima, N. Metzl, F. Millero, D. R. Munro, A. Murata, J. E. M. S. Nabel, S. Nakaoka, Y. Nojiri, K. O'Brien, A. Olsen, T. Ono, F. F. Pérez, B. Pfeil, D. Pierrot, B. Poulter, G. Rehder, C. Rödenbeck, S. Saito, U. Schuster, J. Schwinger, R. Séférian, T. Steinhoff, B. D. Stocker, A. J. Sutton, T. Takahashi, B. Tilbrook, I. T. van der Laan-Luijkx, G. R. van der Werf, S. van Heuven, D. Vandemark, N. Viovy, A. Wiltshire, S. Zaehle, and N. Zeng
Earth Syst. Sci. Data, 7, 349–396, https://doi.org/10.5194/essd-7-349-2015, https://doi.org/10.5194/essd-7-349-2015, 2015
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Accurate assessment of anthropogenic carbon dioxide emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere is important to understand the global carbon cycle, support the development of climate policies, and project future climate change. We describe data sets and a methodology to quantify all major components of the global carbon budget, including their uncertainties, based on a range of data and models and their interpretation by a broad scientific community.
C. Le Quéré, R. Moriarty, R. M. Andrew, G. P. Peters, P. Ciais, P. Friedlingstein, S. D. Jones, S. Sitch, P. Tans, A. Arneth, T. A. Boden, L. Bopp, Y. Bozec, J. G. Canadell, L. P. Chini, F. Chevallier, C. E. Cosca, I. Harris, M. Hoppema, R. A. Houghton, J. I. House, A. K. Jain, T. Johannessen, E. Kato, R. F. Keeling, V. Kitidis, K. Klein Goldewijk, C. Koven, C. S. Landa, P. Landschützer, A. Lenton, I. D. Lima, G. Marland, J. T. Mathis, N. Metzl, Y. Nojiri, A. Olsen, T. Ono, S. Peng, W. Peters, B. Pfeil, B. Poulter, M. R. Raupach, P. Regnier, C. Rödenbeck, S. Saito, J. E. Salisbury, U. Schuster, J. Schwinger, R. Séférian, J. Segschneider, T. Steinhoff, B. D. Stocker, A. J. Sutton, T. Takahashi, B. Tilbrook, G. R. van der Werf, N. Viovy, Y.-P. Wang, R. Wanninkhof, A. Wiltshire, and N. Zeng
Earth Syst. Sci. Data, 7, 47–85, https://doi.org/10.5194/essd-7-47-2015, https://doi.org/10.5194/essd-7-47-2015, 2015
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Carbon dioxide (CO2) emissions from human activities (burning fossil fuels and cement production, deforestation and other land-use change) are set to rise again in 2014.
This study (updated yearly) makes an accurate assessment of anthropogenic CO2 emissions and their redistribution between the atmosphere, ocean, and terrestrial biosphere in order to better understand the global carbon cycle, support the development of climate policies, and project future climate change.
T. G. Bell, W. De Bruyn, C. A. Marandino, S. D. Miller, C. S. Law, M. J. Smith, and E. S. Saltzman
Atmos. Chem. Phys., 15, 1783–1794, https://doi.org/10.5194/acp-15-1783-2015, https://doi.org/10.5194/acp-15-1783-2015, 2015
U. Schuster, A. J. Watson, D. C. E. Bakker, A. M. de Boer, E. M. Jones, G. A. Lee, O. Legge, A. Louwerse, J. Riley, and S. Scally
Earth Syst. Sci. Data, 6, 175–183, https://doi.org/10.5194/essd-6-175-2014, https://doi.org/10.5194/essd-6-175-2014, 2014
D. C. E. Bakker, B. Pfeil, K. Smith, S. Hankin, A. Olsen, S. R. Alin, C. Cosca, S. Harasawa, A. Kozyr, Y. Nojiri, K. M. O'Brien, U. Schuster, M. Telszewski, B. Tilbrook, C. Wada, J. Akl, L. Barbero, N. R. Bates, J. Boutin, Y. Bozec, W.-J. Cai, R. D. Castle, F. P. Chavez, L. Chen, M. Chierici, K. Currie, H. J. W. de Baar, W. Evans, R. A. Feely, A. Fransson, Z. Gao, B. Hales, N. J. Hardman-Mountford, M. Hoppema, W.-J. Huang, C. W. Hunt, B. Huss, T. Ichikawa, T. Johannessen, E. M. Jones, S. D. Jones, S. Jutterström, V. Kitidis, A. Körtzinger, P. Landschützer, S. K. Lauvset, N. Lefèvre, A. B. Manke, J. T. Mathis, L. Merlivat, N. Metzl, A. Murata, T. Newberger, A. M. Omar, T. Ono, G.-H. Park, K. Paterson, D. Pierrot, A. F. Ríos, C. L. Sabine, S. Saito, J. Salisbury, V. V. S. S. Sarma, R. Schlitzer, R. Sieger, I. Skjelvan, T. Steinhoff, K. F. Sullivan, H. Sun, A. J. Sutton, T. Suzuki, C. Sweeney, T. Takahashi, J. Tjiputra, N. Tsurushima, S. M. A. C. van Heuven, D. Vandemark, P. Vlahos, D. W. R. Wallace, R. Wanninkhof, and A. J. Watson
Earth Syst. Sci. Data, 6, 69–90, https://doi.org/10.5194/essd-6-69-2014, https://doi.org/10.5194/essd-6-69-2014, 2014
P. Landschützer, N. Gruber, D. C. E. Bakker, U. Schuster, S. Nakaoka, M. R. Payne, T. P. Sasse, and J. Zeng
Biogeosciences, 10, 7793–7815, https://doi.org/10.5194/bg-10-7793-2013, https://doi.org/10.5194/bg-10-7793-2013, 2013
T. G. Bell, W. De Bruyn, S. D. Miller, B. Ward, K. H. Christensen, and E. S. Saltzman
Atmos. Chem. Phys., 13, 11073–11087, https://doi.org/10.5194/acp-13-11073-2013, https://doi.org/10.5194/acp-13-11073-2013, 2013
U. Schuster, G. A. McKinley, N. Bates, F. Chevallier, S. C. Doney, A. R. Fay, M. González-Dávila, N. Gruber, S. Jones, J. Krijnen, P. Landschützer, N. Lefèvre, M. Manizza, J. Mathis, N. Metzl, A. Olsen, A. F. Rios, C. Rödenbeck, J. M. Santana-Casiano, T. Takahashi, R. Wanninkhof, and A. J. Watson
Biogeosciences, 10, 607–627, https://doi.org/10.5194/bg-10-607-2013, https://doi.org/10.5194/bg-10-607-2013, 2013
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Short summary
This paper describes a near-surface ocean profiler (NSOP) that is deployed from a research vessel. The NSOP is used to sample the top 10 m of the ocean and pumps water back to the research ship for scientific analyses such as for trace gases. The precision in the depth of the seawater collection improves upon previous methods. The NSOP has been used to observe vertical gradients in the upper 5 m for temperature, carbon dioxide and dimethylsulfide.
This paper describes a near-surface ocean profiler (NSOP) that is deployed from a research...
